Colloidal deposits from evaporating sessile droplets: A computationally efficient framework for predicting the final deposit shape

  • Nathan C. J. Coombs
  • , Mykyta V. Chubynsky
  • , James E. Sprittles

Research output: Contribution to journalArticlepeer-review

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Abstract

A modeling framework for the complete evaporation of particle-laden droplets, including touchdown events where the air-liquid interface approaches the substrate, is presented. The inclusion of particle jamming into the model, creating a transition from free advection to an immobile porous plug, is essential to making realistic predictions for the deposit's dimensions. By removing the need to track jammed particle fronts explicitly, as often considered, we are able to run simulations until solute has jammed everywhere in the drop. This allows for valid comparisons with experimental findings on the dried deposit's topography. Our model can also be easily applied to general contact line geometries, allowing us to explore the influence of contact line curvature on the local deposit profile. Published by the American Physical Society 2024
Original languageEnglish
Article number064607
Number of pages21
JournalPhysical Review E
Volume110
Issue number6
Early online date19 Dec 2024
DOIs
Publication statusE-pub ahead of print - 19 Dec 2024

Bibliographical note

Open access CC-BY

Funding

This work was supported by the EPSRC under Grants No. EP/W031426/1, No. EP/S029966/1, and No. EP/P031684/1. The authors also wish to thank Madeleine Moore for providing the data necessary for the benchmark tests shown in Figs. 4 and 12. The data that support the findings of this study are openly available [81]. The numerical code is available open source [82]. This work was supported by the EPSRC under Grants No. EP/W031426/1, No. EP/S029966/1, and No. EP/P031684/1. The authors also wish to thank Madeleine Moore for providing the data necessary for the benchmark tests shown in Figs. and . The data that support the findings of this study are openly available . The numerical code is available open source .

FundersFunder number
Engineering and Physical Sciences Research CouncilEP/W031426/1, EP/S029966/1, EP/P031684/1

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